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Redox Reactions as Donor–Acceptor Reactions

Redox Reactions as Electron and Atom Donor–Acceptor Processes

In this chapter, redox reactions are viewed specifically as donor–acceptor processes. The general idea of redox, as introduced in the parent chapter, is now translated into precise language: Who gives what to whom? and how can this be recognized in concrete reactions?

Electron-Transfer View: Donor and Acceptor

The most compact description of a redox reaction is:

In a redox process, electrons pass from the reductant to the oxidant:
$$
\text{Reductant} \rightarrow \text{Reductant}^{\text{oxidized}} + e^-
$$
$$
\text{Oxidant} + e^- \rightarrow \text{Oxidant}^{\text{reduced}}
$$
Adding these partial processes (later called half-reactions) gives the overall redox reaction.

Key donor–acceptor roles:

This is a donor–acceptor concept fully analogous to the idea that in acid–base reactions, a Brønsted acid donates protons and a Brønsted base accepts protons. Here, however, electrons are the "particles" being donated and accepted.

Example: Reaction Between Zinc and Copper(II) Ions

Consider the reaction of zinc metal with a solution containing copper(II) ions:
$$
\text{Zn (s)} + \text{Cu}^{2+}(\text{aq}) \rightarrow \text{Zn}^{2+}(\text{aq}) + \text{Cu (s)}
$$

Written as electron donor–acceptor steps:

Roles:

The reaction is nothing more than a coupling of these two donor–acceptor processes.

Oxidation as Electron Donation, Reduction as Electron Acceptance

Using the donor–acceptor language:

Thus, oxidation and reduction always occur together: every electron donated must be accepted by something else.

Some typical patterns:

Atom-Transfer View: Oxygen, Hydrogen, and Electron Donors/Acceptors

Historically, oxidation and reduction were recognized in terms of atoms, not electrons. These atom transfers can also be interpreted as donor–acceptor processes.

Oxygen Transfer

In many classical reactions:

Example:
$$
\text{C} + \text{O}_2 \rightarrow \text{CO}_2
$$

Here, carbon behaves as an oxygen acceptor: it accepts oxygen atoms from $\text{O}_2$. On the electron level, carbon is the reducing agent (electron donor) and $\text{O}_2$ is the oxidizing agent (electron acceptor). Thus:

This shows that in many reactions, an oxygen atom donor (like $\text{O}_2$) is simultaneously an electron acceptor.

Hydrogen Transfer

In many inorganic and organic reactions:

Example:
$$
\text{CuO} + \text{H}_2 \rightarrow \text{Cu} + \text{H}_2\text{O}
$$

Interpretation as donor–acceptor processes:

Hydrogen and oxygen transfers are therefore alternative descriptions of underlying electron donor–acceptor processes.

Internal (Disproportionation) and External (Comproportionation) Donor–Acceptor Processes

Donor–acceptor roles do not always involve two different elements or species; sometimes one and the same element participates simultaneously as donor and acceptor in different parts of the system.

Disproportionation: One Species as Both Donor and Acceptor

In a disproportionation reaction, a single species is both oxidized and reduced:

General scheme:
$$
2\,\text{X}^{n+} \rightarrow \text{X}^{(n+1)+} + \text{X}^{(n-1)+}
$$

Example: Disproportionation of hydrogen peroxide in basic solution:
$$
3\text{H}_2\text{O}_2 \rightarrow 2\text{H}_2\text{O} + \text{O}_2
$$

Part of the $\text{H}_2\text{O}_2$ acts as reductant (electron donor), and another part as oxidant (electron acceptor). The same chemical substance simultaneously provides both donor and acceptor roles.

Comproportionation: Two Oxidation States to One Intermediate

In a comproportionation reaction, species in two different oxidation states of the same element react to form an intermediate oxidation state:

General scheme:
$$
\text{X}^{(n-1)+} + \text{X}^{(n+1)+} \rightarrow 2\,\text{X}^{n+}
$$

One species donates electrons, the other accepts them; the product has an intermediate oxidation state. Donor–acceptor roles are thus divided between two different starting species containing the same element.

Electron-Transfer Chains and Redox Mediation

In many reactions, the ultimate electron donor and acceptor are not in direct contact. Instead, electrons are passed stepwise through mediators. Each step is itself a donor–acceptor process.

Example of a chain idea (schematic):
$$
\text{A} \rightarrow \text{B} \rightarrow \text{C}
$$
where:

Here, B plays a dual role:

Such mediator roles are important in many chemical and biological systems (details are treated elsewhere); conceptually, they are sequences of coupled donor–acceptor steps.

Recognizing Donor and Acceptor Roles in Practice

For any given redox reaction, you can systematically identify donor and acceptor roles by:

  1. Assigning oxidation numbers (covered in a later chapter).
  2. Determining which species increases its oxidation number:
    • This species is oxidizedelectron donorreducing agent.
  3. Determining which species decreases its oxidation number:
    • This species is reducedelectron acceptoroxidizing agent.

Even without oxidation numbers, simple clues often exist:

In every case, the essential donor–acceptor nature of a redox process remains:

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